I’m not sure that the material choice is all that important. The main issue will the the thickness increase.
The downside to the UD is that it can be a little more difficult to infuse properly.
If your test laminates were getting a thickness of .048" and the areal weight of the carbon is actually 5.9 oz/yard then you were getting a Vf of 46%. That would be 57% fiber by weight (assuming PAN based carbon). At that same ratio the thickness increase of the added UD carbon would be .064". I think that you will be able to get a Vf of 55%, or better, with the UD which would yield a thickness increase of .054…maybe a little less. 55% Vf would be 66% by weight.
THE ABOVE CALCULATIONS ARE WRONG DUE TO A MATH ERROR ON MY PART. See post #108 for my corrections.